Issue 87, 2021
From the journal:

Chemical Communications

Room-temperature spin nutations in a magnetically condensed phase of [Y(pc)2]˙†

Athanassios K. Boudalis, ORCID logo *abc   Jorge-Enrique Olivares-Peña,a   Eufemio Moreno-Pineda, ORCID logo d   Artem Fediai,a   Wolfgang Wenzel,a   Philippe Turek ORCID logo e  and  Mario Ruben*abc  

* Corresponding authors

a Karlsruhe Institute of Technology (KIT), Institute of Nanotechnology, Eggenstein-Leopoldshafen, Germany
E-mail: mario.ruben@kit.edu, bountalis@unistra.fr

b Institute for Quantum Materials and Technology (IQMT), Karlsruhe Institute of Technology (KIT), Eggenstein-Leopoldshafen, Germany

c Institut de Science et d’Ingénierie Suparamolaiculaires – ISIS, 8 allée Gaspard Monge, BP 70028, Strasbourg Cedex F-67083, France

d Departamento de Química-Física, Escuela de Química, Facultad de Ciencias Naturales, Exactas y Tecnología, Universidad de Panamá, Panama

e Institut de Chimie de Strasbourg (UMR 7177, CNRS-Unistra), Université de Strasbourg, 4 rue Blaise Pascal, CS 90032, Strasbourg F-67081, France

Abstract

FID-detected nutations of the antiferromagnetic crystal form of [Y(pc)2]˙ demonstrated that its radical spin can be coherently driven in its magnetically condensed undeuterated phase and at room temperature. Liquid-helium nutations revealed additional Rabi oscillations assigned to transitions within higher-multiplicity states of finite-sized chain fragments.

Graphical abstract: Room-temperature spin nutations in a magnetically condensed phase of [Y(pc)2]˙

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Article information

DOI
https://doi.org/10.1039/D1CC05491K
Article type
Communication
Submitted
29 Sep 2021
Accepted
10 Oct 2021
First published
11 Oct 2021

Chem. Commun., 2021,57, 11505-11508

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Room-temperature spin nutations in a magnetically condensed phase of [Y(pc)2]˙

A. K. Boudalis, J. Olivares-Peña, E. Moreno-Pineda, A. Fediai, W. Wenzel, P. Turek and M. Ruben, Chem. Commun., 2021, 57, 11505 DOI: 10.1039/D1CC05491K

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