Improving the direct air capture capacity of grafted amines via thermal treatment†
Abstract
This study investigates the effects of elevated temperature thermal treatments on the direct air capture of CO2 by aminosilane-grafted SBA-15 silica sorbents. Exposing samples to high temperatures (200–250 °C compared to 80–120 °C) in an inert environment resulted in improved CO2 capacity (5–21%) that was sustained over multiple adsorption/desorption cycles.