Transparent, mechanically robust, conductive, self-healable, and recyclable ionogels for flexible strain sensors and electroluminescent devices

Abstract

A mechanically robust, self-healable, and recyclable PVP-based ionogel was achieved through a simple one-pot photoinitiated polymerization process. This ionogel exhibits a combination of excellent properties, including transparency, high mechanical strength, good ionic conductivity, self healability, and recyclability. A wearable resistive strain sensor based on the ionogel is successfully assembled and demonstrated accurate response to human motion. Moreover, a flexible electroluminescent device has been fabricated based on our ionogel, which can maintain optimal luminescence functionality even when subjected to bending. Considering the simple preparation method and excellent applications, we believe that our PVP-based ionogel has promising applications in many fields such as in wearable devices, electronic skin, implantable materials, robotics and human–machine interfaces.