Themed collection Editor’s Choice collection: Nanoarchitectonics: fine structure construction in nanoscale


Synthesis and application of polypyrrole nanofibers: a review
Polypyrrole nanofibers are generally synthesized by electrospinning, interfacial polymerization, and template methods, and show advanced functions and a broad range of applications in biomedical engineering, energy storage, and organic electronics.
Nanoscale Adv., 2023,5, 3606-3618
https://doi.org/10.1039/D3NA00138E

Synergistic integration of MXene nanostructures into electrospun fibers for advanced biomedical engineering applications
MXene-based architectures have paved the way in various fields, particularly in the healthcare area, owing to their remarkable physiochemical and electromagnetic characteristics.
Nanoscale Horiz., 2024,9, 1703-1724
https://doi.org/10.1039/D4NH00209A

Bio-gel nanoarchitectonics in tissue engineering
Nanoarchitectonics may be highly compatible with applications in biological systems. Construction strategies and functions of bio-gel nanoarchitectonics in medical applications and tissue engineering are discussed.
Nanoscale, 2024,16, 13230-13246
https://doi.org/10.1039/D4NR00609G

MXenes vs. clays: emerging and traditional 2D layered nanoarchitectonics
Clays and MXenes: comparison and analogies of the preparation, properties and applications of nanoarchitectures based on them.
Nanoscale, 2023,15, 18959-18979
https://doi.org/10.1039/D3NR03037G

Recent advancements in zero- to three-dimensional carbon networks with a two-dimensional electrode material for high-performance supercapacitors
Supercapacitors have gained significant attention owing to their exceptional performance in various applications, such as mobile devices, electric vehicles, and renewable energy storage systems.
Nanoscale Adv., 2023,5, 3146-3176
https://doi.org/10.1039/D3NA00094J
A bioinspired helical hydrogel scaffold with real-time sensing for enhanced precision in gynecological digital vaginal examination
A stent can be wrapped around a physician's finger for gathering real-time clinical data during examinations.
Nanoscale Horiz., 2025,10, 1131-1139
https://doi.org/10.1039/D4NH00636D

Block copolymer-assembled nanopore arrays enable ultrasensitive label-free DNA detection
Block copolymer self-assembly enables precise thin-film materials architectures on electrodes for nanopore blockage-based electrochemical DNA detection. This scalable method achieves 30 fM sensitivity in under 20 minutes, advancing portable and accurate biosensing technologies.
Nanoscale Horiz., 2025,10, 760-769
https://doi.org/10.1039/D4NH00466C
Nanoparticle-assembled interconnected PbO1.44 hollow spheres enabled by PVP-driven transformation of β-PbO2 and self-sacrificial templating for superior lithium storage
Nanoparticle-assembled interconnected PbO1.44 hollow spheres (NAHSs) were crafted by a robust strategy of PVP-driven transformation of β-PbO2 microspheres (MSs) combined with a self-sacrificial templating mechanism for superior lithium storage.
Nanoscale, 2025,17, 3023-3034
https://doi.org/10.1039/D4NR04763J
Surface modification of a biomass-derived self-supported carbon nano network as an emerging platform for advanced field emitter devices and supercapacitor applications
The architecture of self-supported carbon network, which incorporates F doping, the in situ formation of CaF2, and graphitic nanocrystals, contributes to enhanced field emission and electrochemical properties.
Nanoscale Horiz., 2024,9, 2259-2272
https://doi.org/10.1039/D4NH00314D

Template-directed 2D nanopatterning of S = 1/2 molecular spins
We demonstrate fabrication of a surface-supported array of VOPc with controlled spin-spin distance, electronic decoupling from the substrate, and individual addressability to realize molecular qubit platforms interfaceable to solid state devices.
Nanoscale Horiz., 2023,8, 624-631
https://doi.org/10.1039/D2NH00375A

Nanoarchitectonics in fully printed perovskite solar cells with carbon-based electrodes
In this work, we demonstrate a novel nanoarchitectonic approach to tailor perovskite crystal growth leading to the enhancement of the opto-electronic properties and power conversion efficiency of perovskite solar cells.
Nanoscale, 2023,15, 3130-3134
https://doi.org/10.1039/D2NR05856A

Electronic structure tunability of carbon-based 1D-polymers combining cross-conjugation and nitrogen doping
We produce atomically precise cross-conjugated one-dimensional polymeric chains designed in their heteroatom content. The pyridine location and number in the chains effectively tune both the gap size and the frontier orbital energy positions.
Nanoscale, 2025,17, 14827-14836
https://doi.org/10.1039/D5NR01235J

Study on the importance of uniformity and nanoparticle size in ZIF-8 carbon nanoarchitecture for enhancing electrochemical properties
This study aimed to assess the effects of the particle size and uniformity of ZIF-8-C on its effectiveness as a nanoporous carbon platform in electrochemical applications.
Nanoscale, 2025,17, 10344-10355
https://doi.org/10.1039/D5NR00556F
An organic array of quantum corrals modulated by the gold herringbone electronic superlattice
We unveil the modulation of the electronic structure induced by the delicate interplay between the Au(111) herringbone potential and that of an organic array of quantum corrals.
Nanoscale, 2025,17, 10314-10323
https://doi.org/10.1039/D5NR00148J
Design of a new process for the stabilization of FeS–Bi2S3 hybrid nanostructure and its application as a field emitter
Design of a new process for the fabrication of FeS–Bi2S3 anisotropic nanostructure for field emission application.
Nanoscale, 2024,16, 21847-21855
https://doi.org/10.1039/D4NR04138K
Localized three-photon upconversion enhancement in silver nanowire networks and its effect in thermal sensing
Localized enhancement of upconversion luminescence in silver nanowires allows the direct visualization of plasmonic hot-spots; however, the effect on the emission spectra of Er3+ ions must be corrected for accurate ratiometric thermometry analysis.
Nanoscale, 2024,16, 18941-18951
https://doi.org/10.1039/D4NR02484B
2D petal-like PdAg nanosheets promote efficient electrocatalytic oxidation of ethanol and methanol
2D petal-like PdAg nanosheets with ultrathin 2D structure and jagged edges promote efficient electrocatalytic oxidation of ethanol and methanol.
Nanoscale, 2024,16, 14096-14100
https://doi.org/10.1039/D4NR01537A

An integrated design strategy coupling additive manufacturing and matrix-assisted pulsed laser evaporation (MAPLE) towards the development of a new concept 3D scaffold with improved properties for tissue regeneration
New concept 3D scaffolds coated with a biocompatible graphene material (GL) obtained by combining additive manufacturing (AM) and matrix-assisted and pulsed laser evaporation (MAPLE) deposition are potential candidates for bone tissue engineering.
Nanoscale Adv., 2024,6, 3064-3072
https://doi.org/10.1039/D4NA00098F
Nanoarchitectonics composite hydrogels with high toughness, mechanical strength, and self-healing capability for electrical actuators with programmable shape memory properties
Multifunctional composite hydrogels exhibit excellent anti-freezing, moisturising, self-healing, transparency and shape memory properties.
Nanoscale, 2023,15, 18667-18677
https://doi.org/10.1039/D3NR03578F

Engineering endosomolytic nanocarriers of diverse morphologies using confined impingement jet mixing
Confined impingement jet (CIJ) mixing was utilized to fabricate pH-responsive endosomolytic polymeric nanocarriers. Manipulation of polymer and formulation properties facilitated the production of multiple nanocarriers with distinct characteristics.
Nanoscale, 2023,15, 16016-16029
https://doi.org/10.1039/D3NR02874G
Multifunctional metal selenide-based materials synthesized via a one-pot solvothermal approach for electrochemical energy storage and conversion applications
One-pot solvothermal approach was adapted to fabricate iron-nickel seleniede spring-lawn-like hetero-nanoarchitectures for rechargeable energy storage from wind energy in portable electronic applications.
Nanoscale, 2023,15, 13049-13061
https://doi.org/10.1039/D3NR02103C

Atomic-layered V2C MXene containing bismuth elements: 2D/0D and 2D/2D nanoarchitectonics for hydrogen evolution and nitrogen reduction reaction
2D/0D and 2D/2D nanoarchitectonics of V2C/Bi and V2C/BiVO4 is capable to enhance the electrocatalytic activities of HER and NRR.
Nanoscale, 2023,15, 12648-12659
https://doi.org/10.1039/D3NR01144E
Secondary ligand-induced orthogonal self-assembly of silver nanoclusters into superstructures with enhanced NIR emission
We present a secondary ligand-induced orthogonal self-assembly of atomically precise silver nanocluster building blocks into complex superstructures with enhanced emission.
Nanoscale, 2023,15, 11927-11934
https://doi.org/10.1039/D3NR02561F

Histidine–DNA nanoarchitecture as laccase mimetic DNAzymes
We report on the construction of Cu–histidine (His)–DNA hybrids as laccase-mimetic DNAzymes. Cu–His–DNAzymes provide new insights for the systematic construction of tailor-made active sites for biomimetics.
Nanoscale, 2023,15, 10749-10754
https://doi.org/10.1039/D3NR01625K

Nanoarchitectonics on Z-scheme and Mott–Schottky heterostructure for photocatalytic water oxidation via dual-cascade charge-transfer pathways
A face-contact C3N4/m-BiVO4/rGO ternary composite was constructed for excessive surface recombination during water oxidation. Spatial separation of electron–hole pairs occurs, and strong redox potentials are maintained by the Z-scheme electron transfer.
Nanoscale Adv., 2023,5, 3386-3395
https://doi.org/10.1039/D3NA00182B

Langmuir and Langmuir–Blodgett technologies as nanoarchitectonic tools for the incorporation of curcumin in membrane systems
Thermodynamic studies of Langmuir model cell membranes oriented to the rational design of lipid formulations.
Nanoscale, 2023,15, 2891-2903
https://doi.org/10.1039/D2NR06631A
About this collection
Nanoscale Horizons board member, Katsuhiko Ariga (National Institute of Materials Science, Japan) has collated some of the top articles published in Nanoscale Horizons, Nanoscale or Nanoscale Advances related to nanoarchitectonics. The collection brings together some of the latest developments in structural designs of nanomaterials and strategies to create fine structures from the last couple of years.
We hope you enjoy reading the primary research articles and reviews hand-selected to feature in this exciting collection.