This work features first asymmetric Ni-catalyzed reductive coupling of allylic carbonates with aldehydes, which may proceed via allyl-Ni intermediates although Zn was used as the terminal reductant. Moderate to excellent enantiomeric excess was obtained with excellent functional group tolerance.
Z. Tan, X. Wan, Z. Zang, Q. Qian, W. Deng and H. Gong, Chem. Commun., 2014, 50, 3827 DOI: 10.1039/C3CC49859J
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