Themed collection Atmospheric chemistry in cold environments - Topic Highlight

15 items
Open Access Critical Review

Electrical charging of snow and ice in polar regions and the potential impact on atmospheric chemistry

Different processes can lead to high electrical field strengths in snow and ice in polar regions with the potential to initiate free radical processes and a number of other chemical modifications.

Graphical abstract: Electrical charging of snow and ice in polar regions and the potential impact on atmospheric chemistry
Open Access Critical Review

Snow particles physiochemistry: feedback on air quality, climate change, and human health

During the last several decades, numerous researchers have provided evidence that physical and biogeochemical processes at air-snow/ice-water interfaces are very complex, and, in many cases, interlinked.

Graphical abstract: Snow particles physiochemistry: feedback on air quality, climate change, and human health
Open Access Paper

Toxicological evaluation of SVOCs in exhaust emissions from light-duty vehicles using different fuel alternatives under sub-freezing conditions

SVOC toxicity in vehicle exhaust varies by fuel. Stricter diesel regulations haven't reduced toxicity. Gasoline exhaust poses the highest risk, with compressed natural gas and ethanol/gasoline also showing notable toxicity.

Graphical abstract: Toxicological evaluation of SVOCs in exhaust emissions from light-duty vehicles using different fuel alternatives under sub-freezing conditions
Open Access Paper

Immersion ice nucleation of atmospherically relevant lipid particles

Immersion freezing temperatures of substrate-deposited lipid particles depend on solubility and viscosity.

Graphical abstract: Immersion ice nucleation of atmospherically relevant lipid particles
Open Access Paper

The molecular scale mechanism of deposition ice nucleation on silver iodide

Schematic of the proposed deposition ice nucleation mechanism on AgI (0001).

Graphical abstract: The molecular scale mechanism of deposition ice nucleation on silver iodide
Open Access Paper

Atmospheric oxidation impact on sea spray produced ice nucleating particles

Ice nucleating particles (INPs) in sea spray aerosol (SSA) are important for ice formation in clouds over oceans. We found that SSA INP concentrations during a phytoplankton bloom were degraded with exposure to 3 to 8 days of atmospheric oxidation.

Graphical abstract: Atmospheric oxidation impact on sea spray produced ice nucleating particles
Open Access Paper

Resolving the controls over the production and emission of ice-nucleating particles in sea spray

Oceans emit ice-nucleating particles (INPs) which freeze supercooled cloud droplets, modifying clouds. We added dead biomass of three phytoplankton to seawater. Each time, this stimulated INP production in the water and INP emissions in sea spray.

Graphical abstract: Resolving the controls over the production and emission of ice-nucleating particles in sea spray
Open Access Paper

Using coherent X-rays to follow dynamics in amorphous ices

Amorphous ice plays an important role in our overall understanding of water's phase diagram.

Graphical abstract: Using coherent X-rays to follow dynamics in amorphous ices
Open Access Paper

Sensitivity of ice nucleation parameterizations to the variability in underlying ice nucleation rate coefficients

We use simulated droplet freezing experiments to probe the impact of variability in ice nucleation propensities (represented as differently-shaped distributions), and observe differences at low frozen fractions and for broad distributions.

Graphical abstract: Sensitivity of ice nucleation parameterizations to the variability in underlying ice nucleation rate coefficients
Open Access Paper

Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada

Airborne dust from the Kaskawulsh Glacier outwash sediments contains effective INPs. The concentrations and properties of the INPs were investigated.

Graphical abstract: Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada
Open Access Paper

Ice nucleation imaged with X-ray spectro-microscopy

Ice nucleation can now be imaged in situ using X-ray spectro-microscopy in a new experiment, which is applied to mineral aerosol particles composed of ferrihydrite or feldspar and associated organic matter.

Graphical abstract: Ice nucleation imaged with X-ray spectro-microscopy
Open Access Paper

Size-fractionation of trace elements in dusty snow from open pit bitumen mines and upgraders: collection, handling, preparation and analysis of samples from the Athabasca bituminous sands region of Alberta, Canada

A robust sample handling, processing and analytical method was developed for reliable determination of 40 TEs in dusty snow. The “dissolved” TEs in snow from the ABS region were extremely low, and TEs were almost exclusively found in the particulate fraction.

Graphical abstract: Size-fractionation of trace elements in dusty snow from open pit bitumen mines and upgraders: collection, handling, preparation and analysis of samples from the Athabasca bituminous sands region of Alberta, Canada
Open Access Paper

Ice nucleating particles in the Canadian High Arctic during the fall of 2018

Our results suggest that a significant source of ice nucleating particles at Alert, Nunavut, during October and November, was likely ice-free and snow-free land at latitudes >50 °N.

Graphical abstract: Ice nucleating particles in the Canadian High Arctic during the fall of 2018
Open Access Paper

Volcanic ash ice nucleation activity is variably reduced by aging in water and sulfuric acid: the effects of leaching, dissolution, and precipitation

The ice nucleation activity of volcanic ash can change when exposed to liquid water or aqueous sulfuric acid through a complex interplay of geochemical alteration mechanisms.

Graphical abstract: Volcanic ash ice nucleation activity is variably reduced by aging in water and sulfuric acid: the effects of leaching, dissolution, and precipitation
Open Access Paper

Mineral and biological ice-nucleating particles above the South East of the British Isles

Mineral dust is responsible for the ice-nucleating properties of aerosol samples collected over the British Isles below ∼−20 °C, while an additional source, potentially biogenic, must explain the ice-nucleating properties at higher temperatures.

Graphical abstract: Mineral and biological ice-nucleating particles above the South East of the British Isles
15 items

About this collection

Atmospheric chemistry occurring in wintertime and in cold regions can have a unique impact on health, geochemical cycles, and climate, due to the presence of ice clouds, snow, and sea ice. This topic collection highlights important research published in Environmental Science: Atmospheres investigating this exciting area with a particular focus on the characteristics of ice-nucleation events.

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